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Published in

IOP Publishing, Journal of Physics: Condensed Matter, 31(15), p. S2425-S2435

DOI: 10.1088/0953-8984/15/31/317

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A quantitative measure of medium-range order in amorphous materials from transmission electron micrographs

Journal article published in 2003 by R. K. Dash, P. M. Voyles ORCID, J. M. Gibson, M. M. J. Treacy, P. Keblinski
This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

We propose an extension to the technique of fluctuation electron microscopy that quantitatively measures a medium-range order correlation length in amorphous materials. In both simulated images from computer-generated paracrystalline amorphous silicon models and experimental images of amorphous silicon, we find that the spatial autocorrelation function of dark-field transmission electron micrographs of amorphous materials exhibits a simple exponential decay. The decay length measures a nanometre-scale structural correlation length in the sample, although it also depends on the microscope resolution. We also propose a new interpretation of the fluctuation microscopy image variance in terms of fluctuations in local atomic pair distribution functions.