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The Royal Society, Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, 2009(372), p. 20120441, 2014

DOI: 10.1098/rsta.2012.0441

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Strain response of magnetic order in perovskite-type oxide films

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

The role of elastic strain for magnetoelectric materials and devices is twofold. It can induce ferroic orders in thin films of otherwise non-ferroic materials. On the other hand, it provides the most exploited coupling mechanism in two-phase magnetoelectric materials and devices today. Complex oxide films (perovskites, spinels) are promising for both routes. The strain control of magnetic order in complex oxide films is a young research field, and few ab initio simulations are available for magnetic order in dependence on lattice parameters and lattice symmetry. Here, an experimental approach for the evaluation of how elastic strain in thin epitaxial films alters their magnetic order is introduced. The magnetic films are grown epitaxially in strain states controlled by buffer layers onto piezoelectric substrates of 0.72Pb(Mg 1/3 Nb 2/3 )O 3 –0.28PbTiO 3 (001). As an example, the strain dependence of the ordered magnetic moment of SrRuO 3 has been investigated. At a tensile strain level of approximately 1%, SrRuO 3 is tetragonal, and biaxial elastic strain induces a pronounced suppression of the ordered magnetic moment. As a second example, a strain-driven transition from a ferromagnetic to a magnetically disordered phase has been observed in epitaxial La 0.8 Sr 0.2 CoO 3 films.