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Conjugated small molecule hole transport materials (HTMs) with tunable energy levels have been designed and synthesized for efficient perovskite solar cells. A champion device with efficiency of 16.2% has been demonstrated using our dopant-free DERDTS-TBDT HTM, while the DORDTS-DFBT HTM-based device shows an inferior performance of 6.2% due to its low hole mobility and unmatched HOMO level with valence band of perovskite film.