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American Geophysical Union, Journal of Geophysical Research, D9(103), p. 11057-11070, 1998

DOI: 10.1029/97jd02613

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Relationship between chemistry of air, fresh snow and firn cores for aerosol species in coastal Antarctica

Journal article published in 1998 by E. W. Wolff, J. S. Hall, R. Mulvaney ORCID, E. C. Pasteur, D. Wagenbach, M. Legrand
This paper is available in a repository.
This paper is available in a repository.

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Data provided by SHERPA/RoMEO

Abstract

Aerosol and fresh snow concentrations have been determined at three coastal Antarctic stations, Dumont d'Urville, Halley, and Neumayer. Model estimates suggest that dry deposition, including that caused by wind pumping, is only a minor contributor (of order 1%) to chemical fluxes at these sites with relatively high snow accumulation. Larger dry deposition fluxes are possible for very large aerosol particles, including sea-salt aerosol. Measurements of surface snow on successive days provide experimental data that constrain the contribution of dry deposition to probably less than 10% of annual fluxes for all ions, although very high episodic fluxes of giant sea-salt aerosol cannot be ruled out. Spatial variability, and frequent snow, fog and drift events, make it difficult to improve this quantification. Both theory and measurement suggest that fog deposition is also a minor contributor to the annual flux (probably