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IOP Publishing, Journal of Physics: Condensed Matter, 11(21), p. 115902

DOI: 10.1088/0953-8984/21/11/115902

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High tunability of the soft mode in strained SrTiO3/DyScO3multilayers

Journal article published in 2009 by C. Kadlec ORCID, F. Kadlec, H. Němec, P. Kužel, J. Schubert ORCID, G. Panaitov
Distributing this paper is prohibited by the publisher
Distributing this paper is prohibited by the publisher

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Abstract

SrTiO(3)/DyScO(3) epitaxial multilayers with variable number and thickness (10-100 nm) of bilayers deposited on DyScO(3) substrates were investigated by means of time-domain terahertz spectroscopy at room temperature. A tensile strain develops in the SrTiO(3) films and shifts the eigenfrequency of the ferroelectric soft mode down by ∼25-45 cm(-1) with respect to the value found for single crystals. In all films the soft mode strongly hardens upon the electrical bias and a linear coupling to a silent excitation of relaxation type at 10 cm(-1) is observed. We show that the change in the THz and sub-THz response of the layers with an increasing field is determined solely by the soft mode eigenfrequency and we propose a phenomenological model describing the origin of the tunability and the peculiar properties of the ferroelectric soft mode in the terahertz spectral range.