Published in
American Chemical Society, Organic Letters, 10(15), p. 2458-2461, 2013
DOI: 10.1021/ol400926p
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Organocatalyzed Asymmetric Synthesis of Morphans
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Abstract
A general effective organocatalyzed synthesis of enantioenriched morphans with up to 92% ee was developed. The morphan scaffold was constructed in a one-pot tandem asymmetric organocatalyzed Michael addition followed by a domino Robinson annulation/aza-Michael intramolecular reaction sequence from easily available starting materials.