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American Physical Society, Physical review E: Statistical, nonlinear, and soft matter physics, 4(92)

DOI: 10.1103/physreve.92.042504

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Thermo-optical properties and nonlinear optical response of smectic liquid crystals containing gold nanoparticles

This paper is available in a repository.
This paper is available in a repository.

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Abstract

The present work is devoted to the study of the thermo-optical and nonlinear optical properties of smectic samples containing gold nanoparticles with different shapes. By using the time-resolved Z-scan technique, we determine the effects of nanoparticle addition on the critical behavior of the thermal diffusivity and thermo-optical coefficient at the vicinity of the smectic-A-nematic phase transition. Our results reveal that introduction of gold nanoparticles affects the temperature dependence of thermo-optical parameters, due to the local distortions in the orientational order and heat generation provided by guest particles during the laser exposure. Further, we show that a nonlinear optical response may take place at temperatures where the smectic order is well established. We provide a detailed discussion of the effects associated with the introduction gold nanoparticles on the mechanisms behind the thermal transport and optical nonlinearity in liquid-crystal samples. © 2015 American Physical Society.