ISEE Conference Abstracts, 1(2013), p. 4059, 2013
DOI: 10.1289/isee.2013.p-2-08-23
American Chemical Society, Environmental Science and Technology, p. 130904150722005
DOI: 10.1021/es402429h
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Particle number (PN) concentrations (10 - 300 nm in size) were continuously measured over a period of ~45 hours in 56 residences of non-smokers in Copenhagen, Denmark. The highest concentrations were measured when occupants were present and awake (geometric mean, GM: 22.3 × 10^3 cm-3), the lowest when the homes were vacant (GM: 6.1 × 10^3 cm-3) or the occupants were asleep (GM: 5.1 × 10^3 cm-3). Diary entries regarding occupancy and particle related activities were used to identify source events and apportion the daily integrated exposure among sources. Source events clearly resulted in increased PN concentrations and decreased average particle diameter. For a given event, elevated particle concentrations persisted for several hours after the emission of fresh particles ceased. The residential daily integrated PN exposure in the 56 homes ranged between 37 × 10^3 and 6.0 × 10^6 particles per cm3•h/day (GM: 3.3 × 10^5 cm-3•h/day). On average, ~90% of this exposure occurred outside of the period from midnight to 6 AM. Source events, especially candle burning, cooking, toasting and unknown activities, were responsible on average for ~65% of the residential integrated exposure (51% without the unknown activities). Candle burning occurred in half of the homes where, on average, it was responsible for almost 60% of the integrated exposure.