Dissemin is shutting down on January 1st, 2025

Published in

Nature Research, Nature Communications, 1(5), 2014

DOI: 10.1038/ncomms6823

Links

Tools

Export citation

Search in Google Scholar

Evolution of hidden localized flow during glass-to-liquid transition in metallic glass

Journal article published in 2014 by Z. Wang ORCID, B. A. Sun, H. Y. Bai ORCID, W. H. Wang
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

Full text: Download

Green circle
Preprint: archiving allowed
Red circle
Postprint: archiving forbidden
Green circle
Published version: archiving allowed
Data provided by SHERPA/RoMEO

Abstract

For glasses, the structural origin of their flow phenomena, such as elastic and plastic deformations especially the microscopic hidden flow before yield and glass-to-liquid transition, is unclear yet due to the lack of structural information. Here we investigate the evolution of the microscopic localized flow during glass-to-liquid transition in a prototypical metallic glass combining with dynamical mechanical relaxations, temperature-dependent tensile experiments and stress relaxation spectra. We show that the unstable and high mobility nano-scale liquid-like regions acting as flow units persist in the glass and can be activated by either temperature or external stress. The activation of such flow units is initially reversible and correlated with β-relaxation. As the proportion of the flow units reaches a critical percolation value, a mechanical brittle-to-ductile transition or macroscopic glass-to-liquid transition happens. A comprehensive picture on the hidden flow as well as its correlation with deformation maps and relaxation spectrum is proposed.