Elsevier, Journal of Alloys and Compounds, (640), p. 462-467, 2015
DOI: 10.1016/j.jallcom.2015.03.215
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We report on the effect of an applied static magnetic field on the dielectric properties of ferroelectric relaxor/ferrimagnetic composites consisting of [Ba(Sn0.3Ti0.7)O3]0.8–[CoFe2O4]0.2 (BST0.8–CFO0.2). The pure Ba(Sn0.3Ti0.7)O3 (BST30) as well as the composites, were synthesized by solid state reaction method. The X-ray diffraction analysis confirmed that BST30 and CFO coexist in the composite without any secondary phase. The real and the imaginary part of the dielectric permittivity were studied as a function of temperature, with and without static magnetic field, respectively. Relaxor characteristics such as dielectric permittivity and its peak temperature are observed to vary with the magnetic field. This is explained in the context that the applied magnetic field creates magnetostriction in the ferrite phase which is transferred to the relaxor phase via the interface coupling. The strain in the relaxor phase results in the reorientation of local polarization entities, polar nano regions (PNRs), which alters the dielectric characteristics of the sample. This effect is explained in relation to local order parameter q(T) which is found to increase in a certain temperature range above the typical ferroelectric temperature regime with the application of magnetic field.