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Elsevier, Physica B: Condensed Matter, (312-313), p. 906-908

DOI: 10.1016/s0921-4526(01)01212-1

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Magnetic properties of U(Ga1−xMx)2 with M=Cu, Al and Ge

Journal article published in 2002 by L. M. da Silva, F. G. Gandra, D. P. Rojas, L. P. Cardoso, A. N. Medina ORCID
This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

We report on magnetization measurements on U(Ga1−xMx)2, M=Cu, Ge and Al, with 0⩽x⩽0.2. All studied samples are ferromagnetic and the magnetization at low field depends on the sample history. Substitution of Cu for Ga strongly shifts Tc to lower temperatures (79K for x=0.1) and induces the formation of a spin-glass phase above x=0.2. The Al- and Ge-doped samples present only a small reduction of Tc reaching 118K for x=0.1. Our results are not explained by the unit cell volume behavior, and indicate that the electronic configuration of the non-f element is responsible for the magnetic properties of this system. The observed reduction of the effective moment indicate that the Uranium moment becomes more delocalized for the Cu- and Ge-doped samples when compared to U(Ga,Al)2.