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American Physical Society, Physical Review Letters, 8(92), 2004

DOI: 10.1103/physrevlett.92.087202

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Orbital Ordering in L a 0.5 S r 1.5 M n O 4 Studied by Soft X-Ray Linear Dichroism

This paper is available in a repository.
This paper is available in a repository.

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Abstract

We found that the conventional model of orbital-ordering of 3x(2)-r(2)/3y(2)-r(2) type in the e(g) states of La0.5Sr1.5MnO4 is incompatible with measurements of linear dichroism in the Mn 2p-edge x-ray absorption, whereas these e(g) states exhibit predominantly cross-type orbital ordering of x(2)-z(2)/y(2)-z(2). LDA+U band-structure calculations reveal that such a cross-type orbital-ordering results from a combined effect of antiferromagnetic structure, Jahn-Teller distortion, and on-site Coulomb interactions.