Published in

American Chemical Society, Journal of Physical Chemistry B (Soft Condensed Matter and Biophysical Chemistry), 24(118), p. 6908-6914, 2014

DOI: 10.1021/jp5034917

Links

Tools

Export citation

Search in Google Scholar

Graphene Sculpturene Nanopores for DNA Nucleobase Sensing

This paper is available in a repository.
This paper is available in a repository.

Full text: Download

Green circle
Preprint: archiving allowed
  • Must obtain written permission from Editor
  • Must not violate ACS ethical Guidelines
Orange circle
Postprint: archiving restricted
  • Must obtain written permission from Editor
  • Must not violate ACS ethical Guidelines
Red circle
Published version: archiving forbidden
Data provided by SHERPA/RoMEO

Abstract

To demonstrate the potential of nanopores in bilayer graphene for DNA sequencing, we compute the current-voltage characteristics of a bilayer graphene junction containing a nanopore and show that this changes significantly when nucleobases are transported through the pore. To demonstrate the sensitivity and selectivity of exemplar devices, we compute the probability distribution Px(β) of the quantity β representing the change in the logarithmic current through the pore due to the presence of a nucleobase X (= adenine, thymine, guanine or cytosine). We quantify the selectivity of the bilayer-graphene nanopores by showing that Px(β) possesses distinct peaks for each base X. To demonstrate that such discriminating sensing is a general feature of bilayer nanopores, the well-separated positions of these peaks are shown to be present for different pores, with alternative examples of electrical contacts.