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Tandem 4+3 cycloaddition/nucleophilic trapping reactions of butyne-1,4-diether dicobalt hexacarbonyl complexes

Journal article published in 2001 by Yafan Lu, James R. Green ORCID
This paper was not found in any repository; the policy of its publisher is unknown or unclear.
This paper was not found in any repository; the policy of its publisher is unknown or unclear.

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Abstract

Butyne-1,4-diether hexacarbonyldicobalt complexes 1 undergo Lewis acid mediated 4+3 cycloadditions with allylsilanes, incorporating halide from the Lewis acid to give halocycloheptynes 3, 6, 7. A phenyl group may be incorporated in place of the halogen (to give 8) by use of benzene as solvent and with B(C6F5)(3) as the Lewis acid; chlorobenzene and toluene also participate in the process.