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American Chemical Society, Nano Letters, 8(15), p. 5455-5464, 2015

DOI: 10.1021/acs.nanolett.5b01849

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High-Efficiency All-Solution-Processed Light-Emitting Diodes Based on Anisotropic Colloidal Heterostructures with Polar Polymer Injecting Layers

Journal article published in 2015 by Andrea Castelli, Francesco Meinardi, Mariacecilia Pasini, Francesco Galeotti, Valerio Pinchetti, Monica Lorenzon, Liberato Manna, Iwan Moreels, Umberto Giovanella, Sergio Brovelli ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Colloidal quantum dots (QDs) are emerging as true candidates for light-emitting diodes with ultrasaturated colors. Here, we combine CdSe/CdS dot-in-rod heterostructures and polar/polyelectrolytic conjugated polymers to demonstrate the first example of fully solution-based quantum dot light-emitting diodes (QD-LEDs) incorporating all-organic injection/transport layers with high brightness, very limited roll-off and external quantum efficiency as high as 6.1%, which is 20 times higher than the record QD-LEDs with all-solution-processed organic interlayers and exceeds by over 200% QD-LEDs embedding vacuum-deposited organic molecules.