Published in

MDPI, Nanomaterials, 8(14), p. 707, 2024

DOI: 10.3390/nano14080707

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Pump-Driven Opto-Magnetic Properties in Semiconducting Transition-Metal Dichalcogenides: An Analytical Model

Journal article published in 2024 by Habib Rostami ORCID, Federico Cilento ORCID, Emmanuele Cappelluti ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Single-layer transition-metal dichalcogenides provide an unique intrinsic entanglement between the spin/valley/orbital degrees of freedom and the polarization of scattered photons. This scenario gives rise to the well-assessed optical dichroism observed by using both steady and time-resolved probes. In this paper, we provide compact analytical modeling of the onset of a finite Faraday/Kerr optical rotation upon shining with circularly polarized light. We identify different optical features displaying optical rotation at different characteristic energies, and we describe in an analytical framework the time-dependence of their intensities as a consequence of the main spin-conserving and spin-flip processes.