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MDPI, Magnetochemistry, 5(9), p. 115, 2023

DOI: 10.3390/magnetochemistry9050115

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Effect of Co-Doping on the Magnetic Ground State of the Heavy-Fermion System CeCu2Ge2 Studied by Neutron Diffraction

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

The antiferromagnetic phase transition of the heavy-fermion system Ce(Cu1−xCox)2Ge2 for x = 0.05 and 0.2, showing up in specific heat, magnetic susceptibility, and muon spin relaxation (μSR) data, has been further investigated. The neutron diffraction (ND) results show that Co-doping drastically reduces the moment size of Ce, without a qualitative change in the magnetic structure of the undoped compound CeCu2Ge2. An incommensurate magnetic propagation vector k = (0.2852, 0.2852, 0.4495) with a cycloidal magnetic structure with a Ce moment of 0.55 μB in the ab-plane has been observed for x = 0.05. Although for x = 0.2 the specific heat and magnetic susceptibility data reflect a phase transition with a broad peak and the muon relaxation rate shows a sharp peak at T = 0.9 K, our ND data dismiss the possibility of a long-range magnetic ordering down to 50 mK. The ND data, along with previously reported results for x = 0.2, are interpreted in terms of the reduced ordered state magnetic moments of the Ce3+ ion by Kondo screening and the presence of dynamical short-range magnetic correlations.