Soils play a key role in meeting the UN Sustainable Development Goals (SDGs). In this study, we review the contribution of soils to the regulation of air quality, which is one of ‘Nature's Contributions to People’ identified by the Intergovernmental-Policy Platform on Biodiversity and Ecosystem Services (IPBES). This is particularly relevant for SDG3 (health and well-being) and 11 (sustainable cities and well-being) but also impacts other SDGs. Soils can act as both a source and a sink of air pollutants (and their precursors). In addition, soils support plant growth which plays a major role in regulating air quality. The scale of the soil impacts on air quality range from global (e.g. greenhouse gas fluxes, stratospheric ozone depletion) to local (e.g. odours, particulates, pathogen transport). Harmful emissions from soil can be increased or decreased by anthropogenic activity, while climate change is likely to modify future emissions patterns, both directly and in response to human mitigation and adaption actions. Although soils are not the only source of these pollutants, it is worthwhile managing them to reduce erosion and nutrient losses to maintain soil health so we may continue to benefit from the contributions to good quality of life they provide. This article is part of the theme issue ‘The role of soils in delivering Nature's Contributions to People’.