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National Academy of Sciences, Proceedings of the National Academy of Sciences, 40(118), 2021

DOI: 10.1073/pnas.2023337118

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Topological spin/structure couplings in layered chiral magnet Cr <sub>1/3</sub> TaS <sub>2</sub> : The discovery of spiral magnetic superstructure

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Significance Magnets in which chirality of crystal lattice gives rise to noncollinear spin orders are ideal playgrounds for studies of novel physical phenomena originating from the nontrivial topology of magnetic textures. Most studies have been focused on homochiral materials, while topological magnetic states of heterochiral magnets have rarely been explored. Here, we report a layered chiral helimagnet with highly tunable topological heterochiral states. Tuning the chiral domain density, we have observed a topological magnetic texture that has the form of a spiral unfolding in the radial direction. In weak in-plane fields, this spiral magnetic superstructure transforms into a nonspiral array of concentric rings. Our results open a horizon for studies of tunable topological magnetic textures.