Published in

Nature Research, Nature Communications, 1(13), 2022

DOI: 10.1038/s41467-022-30829-z

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Slowdown of photoexcited spin dynamics in the non-collinear spin-ordered phases in skyrmion host GaV4S8

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

AbstractFormation of magnetic order alters the character of spin excitations, which then affects transport properties. We investigate the photoexcited ultrafast spin dynamics in different magnetic phases in Néel-type skyrmion host GaV4S8 with time-resolved magneto-optical Kerr effect experiments. The coherent spin precession, whose amplitude is enhanced in the skyrmion-lattice phase, shows a signature of phase coexistence across the magnetic phase transitions. The incoherent spin relaxation dynamics slows down by a factor of two in the skyrmion-lattice/cycloid phases, indicating significant decrease in thermal conductivity triggered by a small change of magnetic field. The slow heat diffusion in the skyrmion-lattice/cycloid phases is attributed to the stronger magnon scattering off the domain walls formed in abundance in the skyrmion-lattice/cycloid phase. These results highlight the impact of spatial spin structure on the ultrafast heat transport in spin systems, providing a useful insight for the step toward ultrafast photocontrol of the magnets with novel spin orders.