Published in
The International Conference on Ultrafast Phenomena (UP) 2022, 2022
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From Femtosecond Excited-State and Dissociation Dynamics to Nanosecond Reaction Kinetics: Following C-H Bond Activation with X-rays
Proceedings article published in 2022 by
Raphael M. Jay,
Ambar Banerjee 
,
Torsten Leitner,
Robert Stefanuik,
Ru-Pan Wang,
Jessica Harich,
Emma Beale,
Victoria Kabanova,
Abdullah Kahraman,
Anna Wach,
Dimitri Ozerov,
Christopher A. Arrell,
Philip J. M. Johnson,
Grigory Smolentsev,
Thomas Huthwelker
and other authors.
,
Torsten Leitner,
Robert Stefanuik,
Ru-Pan Wang,
Jessica Harich,
Emma Beale,
Victoria Kabanova,
Abdullah Kahraman,
Anna Wach,
Dimitri Ozerov,
Christopher A. Arrell,
Philip J. M. Johnson,
Grigory Smolentsev,
Thomas Huthwelker
and other authors.
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Abstract
Using ultrafast X-ray absorption spectroscopy, we observe how a rhodium carbonyl catalyst is formed on femtosecond timescales and reveal the decisive orbital interactions which facilitate the efficient cleavage of an alkane C-H bond from solution.