AbstractThe recently emerged ferromagnetic two-dimensional (2D) materials provide unique platforms for compact spintronic devices down to the atomic-thin regime; however, the prospect is hindered by the limited number of ferromagnetic 2D materials discovered with limited choices of magnetic properties. If 2D antiferromagnetism could be converted to 2D ferromagnetism, the range of 2D magnets and their potential applications would be significantly broadened. Here, we discovered emergent ferromagnetism by interfacing non-magnetic WS₂ layers with the antiferromagnetic FePS₃. The WS₂ exhibits an order of magnitude enhanced Zeeman effect with a saturated interfacial exchange field ~38 Tesla. Given the pristine FePS₃ is an intralayer antiferromagnet, the prominent interfacial exchange field suggests the formation of ferromagnetic FePS₃ at interface. Furthermore, the enhanced Zeeman effect in WS₂ is found to exhibit a strong WS₂-thickness dependence, highlighting the layer-tailorable interfacial exchange coupling in WS₂-FePS₃ heterostructures, which is potentially attributed to the thickness-dependent interfacial hybridization.