Abstract The NWS/NCEP recently implemented a new global deterministic aerosol forecast model named the Global Ensemble Forecast Systems Aerosols (GEFS-Aerosols), which is based on the Finite Volume version 3 GFS (FV3GFS). It replaced the operational NOAA Environmental Modeling System (NEMS) GFS Aerosol Component version 2 (NGACv2), which was based on a global spectral model (GSM). GEFS-Aerosols uses aerosol modules from the GOCART previously integrated in the WRF Model with Chemistry (WRF-Chem), FENGSHA dust scheme, and several other updates. In this study, we have extensively evaluated aerosol optical depth (AOD) forecasts from GEFS-Aerosols against various observations over a timespan longer than one year (2019–20). The total AOD improvement (in terms of seasonal mean) in GEFS-Aerosols is about 40% compared to NGACv2 in the fall and winter season of 2019. In terms of aerosol species, the biggest improvement came from the enhanced representation of biomass burning aerosol species as GEFS-Aerosols is able to capture more fire events in southern Africa, South America, and Asia than its predecessor. Dust AODs reproduce the seasonal variation over Africa and the Middle East. We have found that correlation of total AOD over large regions of the globe remains consistent for forecast days 3–5. However, we have found that GEFS-Aerosols generates some systematic positive biases for organic carbon AOD near biomass burning regions and sulfate AOD over prediction over East Asia. The addition of a data assimilation capability to GEFS-Aerosols in the near future is expected to address these biases and provide a positive impact to aerosol forecasts by the model. Significance Statement The purpose of this study is to quantify improvements associated with the newly implemented global aerosol forecast model at NWS/NCEP. The monthly and seasonal variations of AOD forecasts of various aerosol regimes are overall consistent with the observations. Our results provide a guide to downstream regional air quality models like CMAQ that will use GEFS-Aerosols to provide lateral boundary conditions.