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arXiv, 2022

DOI: 10.48550/arxiv.2206.01286

American Chemical Society, Nano Letters, 16(22), p. 6716-6723, 2022

DOI: 10.1021/acs.nanolett.2c02124

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Anisotropic Gigahertz Antiferromagnetic Resonances of the Easy-Axis van der Waals Antiferromagnet CrSBr

This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

We report measurements of antiferromagnetic resonances in the van der Waals easy-axis antiferromagnet CrSBr. The interlayer exchange field and magnetocrystalline anisotropy fields are comparable to laboratory magnetic fields, allowing a rich variety of gigahertz-frequency dynamical modes to be accessed. By mapping the resonance frequencies as a function of the magnitude and angle of applied magnetic field we identify the different regimes of antiferromagnetic dynamics. The spectra show good agreement with a Landau-Lifshitz model for two antiferromagnetically-coupled sublattices, accounting for inter-layer exchange and triaxial magnetic anisotropy. Fits allow us to quantify the parameters governing the magnetic dynamics: at 5 K, the interlayer exchange field is $μ_0 H_E =$ 0.395(2) T, and the hard and intermediate-axis anisotropy parameters are $μ_0 H_c =$ 1.30(2) T and $μ_0 H_a =$ 0.383(7) T. The existence of within-plane anisotropy makes it possible to control the degree of hybridization between the antiferromagnetic resonances using an in-plane magnetic field.