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American Physical Society, Physical Review Letters, 10(102)

DOI: 10.1103/physrevlett.102.105502

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Transverse Acoustic Excitations in Liquid Ga

This paper is available in a repository.
This paper is available in a repository.

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Abstract

The transverse acoustic excitation modes were detected by inelastic x-ray scattering in liquid Ga in the Q range above 9 nm(-1) although liquid Ga is mostly described by a hard-sphere liquid. An ab initio molecular dynamics simulation clearly supports this finding. From the detailed analysis for the S(Q,omega) spectra with a good statistic quality, the lifetime of 0.5 ps and the propagating length of 0.4-0.5 nm can be estimated for the transverse acoustic phonon modes, which may correspond to the lifetime and size of cages formed instantaneously in liquid Ga.