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Royal Society of Chemistry, Chemical Science, 6(12), p. 2231-2241, 2021

DOI: 10.1039/d0sc06466a

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Activation of Ammonia and Hydrazine by Electron Rich Fe(II) Complexes Supported by a Dianionic Pentadentate Ligand Platform Through a Common Terminal Fe(III) Amido Intermediate

Journal article published in 2021 by Lucie Nurdin, Yan Yang, Peter G. N. Neate, Warren E. Piers ORCID, Maron Laurent, Michael L. Neidig, Jian-Bin Lin, Benjamin Sidney Gelfand ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Synopsis: a highly reactive Fe(iii)–NH2 complex is generated via activation of ammonia or hydrazine in reactions of relevance to fundamental steps in ammonia oxidation processes mediated by an abundant, first row transition metal.