Abstract Voltage-tunable RF/microwave devices attract great attention due to their low power consumption; however, they still suffer from the fundamental dilemma between large tunability and low insertion loss. In this paper, yttrium iron garnet (YIG) polycrystalline thin films with low microwave loss (<3 × 10⁻⁴) were directly deposited on mica substrates via a van der Waals force and then transferred onto PMN-PT substrates. The in-plane magnetic anisotropy of YIG was tuned by the in-plane biaxial stress of PMN-PT, and an improved voltage tunability (175 MHz) of in-plane FMR f_r was obtained due to the removal of the substrate clamping effect. Moreover, our samples still represent good frequency stability (4–12 GHz) during the tuning process. It is of significance for exploiting novel, portable, low-loss RF/microwave devices in the future.