Accurately mapping forest effective leaf area index (LAIe) at the landscape level is a crucial step to better simulate various ecological and physiological processes such as photosynthesis, respiration, transpiration, and precipitation interception. The LAIe products obtained from two-dimensional (2-D) remotely sensed optical imageries are usually biased due to their inability to identify the vertical forest structure and eliminate the effects of forest background (i.e., shrubs, grass, snow, and bare earth). In this study, we first stratified the forest overstory and background layers and generated a forest background mask layer based on the structural information implicitly contained within the aerial laser scanning (ALS) data. We improved the retrieval accuracy of LAIe by combining light detection and ranging (Lidar)-based three dimensional (3-D) structural and 2-D spectral information. Then, we obtained the improved final LAIe estimation result by masking the forest background pixels from the optical remotely sensed imageries. Our results showed that: (1) Removing forest background information could effectively (R2 increase from 20% to 30%) improve the estimation accuracy of optical-based forest LAIe depending on forest structure characteristics. (2) The forest background in the forest stands with low canopy cover showed more apparent effects on LAIe estimation compared with the forest stands with a high canopy cover. (3) The combination of ALS and optical remotely sensed data could produce the best LAIe retrieval result effectively by removing the forest background information.