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Nature Research, Scientific Reports, 1(9), 2019

DOI: 10.1038/s41598-019-49654-4

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Anisotropic magnetocaloric effect in Fe3−xGeTe2

Journal article published in 2019 by Yu Liu ORCID, Jun Li, Jing Tao, Yimei Zhu, Cedomir Petrovic ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

AbstractWe present a comprehensive study on anisotropic magnetocaloric porperties of the van der Waals weak-itinerant ferromagnet Fe3−xGeTe2 that features gate-tunable room-temperature ferromagnetism in few-layer device. Intrinsic magnetocrystalline anisotropy is observed to be temperature-dependent and most likely favors the long-range magnetic order in thin Fe3−xGeTe2 crsytal. The magnetic entropy change ΔSM also reveals an anisotropic characteristic between H//ab and H//c, which could be well scaled into a universal curve. The peak value $-Δ {S}_{M}^{{\max }}$−ΔSMmax of 1.20 J kg−1 K−1 and the corresponding adiabatic temperature change ΔTad of 0.66 K are deduced from heat capacity with out-of-plane field change of 5 T. By fitting of the field-dependent parameters of $-Δ {S}_{M}^{{\max }}$−ΔSMmax and the relative cooling power RCP, it gives $-{\rm{\triangle }}{S}_{M}^{{\max }}$−∆SMmax ∝ Hn with n = 0.603(6) and RCP ∝ Hm with m = 1.20(1) when H//c. Given the high and tunable Tc, Fe3−xGeTe2 crystals are of interest for fabricating the heterostructure-based spintronics device.