National Academy of Sciences, Proceedings of the National Academy of Sciences, 51(114), p. 13380-13384, 2017
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Significance Water provides an attractive medium for storing solar energy via water splitting. Charge-separated states generated by solar capture may be transferred to catalysts that split water to hydrogen and oxygen. Most water-splitting catalysts comprising earth-abundant elements are susceptible to corrosion when operated in neutral and natural water. Such corrosion may be circumvented if the catalysts are self-healing. The design of self-healing catalysts allows neutral water and natural water sources to be used for water splitting, greatly simplifying the implementation of using water as a distributed energy storage medium for solar energy.