Hydrodynamic instabilities and asymmetries are a major obstacle in the quest to achieve ignition at the National Ignition Facility (NIF) as they cause pre-existing capsule perturbations to grow and ultimately quench the fusion burn in experiments. This paper reviews the development of two new experimental techniques to measure high-mode instabilities and low-mode asymmetries in the deceleration phase of indirect drive inertial confinement fusion implosions. In the first innovative technique, self-emission from the hot spot was enhanced with an argon dopant to “self-backlight” the shell in-flight, imaging the perturbations in the shell near peak velocity. Experiments with pre-imposed two-dimensional perturbations showed hydrodynamic instability growth of up to 7000× in areal density. These experiments discovered unexpected three-dimensional structures originating from the capsule support structures. These new 3-D structures became one of the primary concerns for the indirect drive ICF program that requires their origin to be understood and their impact mitigated. In a second complementary technique, the inner surface of the decelerating shell was visualized in implosions using x-ray emission of a high-Z dopant added to the inner surface of the capsule. With this technique, low mode asymmetry and high mode perturbations, including perturbations seeded by the gas fill tube and capsule support structure, were quantified near peak compression. Using this doping method, the role of perturbations and radiative losses from high atomic number materials on neutron yield was quantified.