American Institute of Physics, Applied Physics Letters, 18(109), p. 183901
DOI: 10.1063/1.4966893
Full text: Unavailable
Plasmonic nanostructures have been widely applied in various types of solar cells for improving light absorption and therefore energy conversion efficiency. In this work, we demonstrate that Au@SiO2 core-shell nanorods with finely tuned aspect ratios are highly beneficial for the CH3NH3PbI3 perovskite solar cell, with the simultaneous enhancement of solar absorption and external quantum efficiency across a broad range of wavelength, which can contribute to the increased cross-sectional scattering and spectrally absorbing energy density. Therefore, a 16.1% improvement (from 12.4% to 14.4%) of the maximal external quantum efficiency can be achieved by such structures, accompanied with a 13.5% improvement (from 20.0 to 22.7 mA/cm2) of the maximal short-circuit current density and little improvement of the open-circuit voltage and fill factor. Our findings also provide a general guideline to design solar cell structures with thinner absorber layers and improve the absorption in other poorly light-absorbing devices like lead free perovskite solar cells as well.