Published in

National Academy of Sciences, Proceedings of the National Academy of Sciences, 19(115), p. 4845-4850, 2018

DOI: 10.1073/pnas.1722063115

Links

Tools

Export citation

Search in Google Scholar

Two-dimensional infrared spectroscopy of vibrational polaritons

This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

Full text: Unavailable

Red circle
Preprint: archiving forbidden
Green circle
Postprint: archiving allowed
Red circle
Published version: archiving forbidden
Data provided by SHERPA/RoMEO

Abstract

Significance Quantum states of molecular vibrational polaritons, hybrid half-light, half-matter quasi-particles, are studied using ultrafast coherent two-dimensional infrared spectroscopy. Valuable physical insights such as existence of hidden dark states and ultrafast interactions between dark states and bright polariton states are unambiguously revealed. These results not only advance coherent two-dimensional spectroscopy, but also have significant implications in harvesting the creation of molecular vibrational polaritons for infrared photonic devices, lasing, molecular quantum simulation, as well as chemistry by tailoring potential energy landscapes.