Published in

European Geosciences Union, Atmospheric Chemistry and Physics, 18(18), p. 13345-13361, 2018

DOI: 10.5194/acp-18-13345-2018

European Geosciences Union, Atmospheric Chemistry and Physics Discussions, p. 1-25

DOI: 10.5194/acp-2017-1191

Links

Tools

Export citation

Search in Google Scholar

Observed aerosol suppression of cloud ice in low-level Arctic mixed-phase clouds

Journal article published in 2018 by Matthew S. Norgren, Gijs de Boer ORCID, Matthew D. Shupe ORCID
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

Full text: Download

Green circle
Preprint: archiving allowed
Green circle
Postprint: archiving allowed
Green circle
Published version: archiving allowed
Data provided by SHERPA/RoMEO

Abstract

Abstract. The interactions that occur between aerosols and a mixed-phase cloud system, and the subsequent alteration of the microphysical state of such clouds, are a problem that has yet to be well constrained. Advancing our understanding of aerosol–ice processes is necessary to determine the impact of natural and anthropogenic emissions on Earth's climate and to improve our capability to predict future climate states. This paper deals specifically with how aerosols influence ice mass production in low-level Arctic mixed-phase clouds. In this study, a 9-year record of aerosol, cloud and atmospheric state properties is used to quantify aerosol influence on ice production in mixed-phase clouds. It is found that mixed-phase clouds present in a clean aerosol state have higher ice water content (IWC) by a factor of 1.22 to 1.63 at cloud base than do similar clouds in cases with higher aerosol loading. We additionally analyze radar-derived mean Doppler velocities to better understand the drivers behind this relationship, and we conclude that aerosol induced reduction of the ice crystal nucleation rate, together with decreased riming rates in polluted clouds, are likely influences on the observed reductions in IWC.