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American Institute of Physics, Applied Physics Letters, 20(110), p. 202406

DOI: 10.1063/1.4983810

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Variable-temperature inelastic light scattering spectroscopy of nickel oxide: Disentangling phonons and magnons

This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

We report the results of an investigation of the temperature dependence of the magnon and phonon frequencies in NiO. A combination of Brillouin-Mandelstam and Raman spectroscopies allowed us to elucidate the evolution of the phonon and magnon spectral signatures from the Brillouin zone center (GHz range) to the second-order peaks from the zone boundary (THz range). The temperature-dependent behavior of the magnon and phonon bands in the NiO spectrum indicates the presence of antiferromagnetic (AF) order fluctuation or a persistent AF state at temperatures substantially above the Néel temperature (TN=523 K). Tuning the intensity of the excitation laser provides a method for disentangling the features of magnons from acoustic phonons in AF materials without the application of a magnetic field. Our results are useful for the interpretation of the inelastic-light scattering spectrum of NiO and add to the knowledge of its magnon properties important for THz spintronic devices.