Three-dimensional (3D) nanoworm-like MoS2 architectures have been successfully synthesized and directly supported on graphene foam/carbon nanotubes (GF/CNT) hybrid films. The sp2-hybridized GF/CNT films provide robust frameworks with ideal contact for the nucleation and subsequent massive growth of MoS2 architectures, while act as an efficient current collector with conductive contact for binder-free electrodes. The as-prepared hierarchical MoS2@GF/CNT electrode shows capacities of 1368 mAh g-1 and 823 mAh g-1 at current densities of 200 mA g-1 and 5000 mA g-1, which can retain 81.3% of the initial reversible capacity up to 120 cycles.