The land surface albedo in the NCAR Community Climate System Model (CCSM2) is calculated based on a two-stream approximation, which does not include the effect of three-dimensional vegetation structure on radiative transfer. The model albedo (including monthly averaged albedo, direct albedo at local noon, and the solar zenith angle dependence of albedo) is evaluated using the Moderate Resolution Imaging Spectroradiometer (MODIS) Bidirectional Reflectance Distribution Function (BRDF) and albedo data acquired during July 2001-July 2002. The model monthly averaged albedos in February and July are close to the MODIS white-sky albedos (within 0.02 or statistically insignificant) over about 40% of the global land between 60°S and 70°N. However, CCSM2 significantly underestimates albedo by 0.05 or more over deserts (e.g., the Sahara Desert) and some semiarid regions (e.g., parts of Australia). The difference between the model direct albedo at local noon and the MODIS black-sky albedo for the near-infrared (NIR) band (with wavelength > 0.7 μm) is larger than the difference for the visible band (with wavelength < 0.7 μm) for most snow-free regions. For eleven model grid cells with different dominant plant functional types, the model diffuse NIR albedo is higher by 0.05 or more than the MODIS white-sky albedo in five of these cells. Direct albedos from the model and MODIS (as computed using the BRDF parameters) increase with solar zenith angles, but model albedo increases faster than the MODIS data. These analyses and the MODIS BRDF and albedo data provide a starting point toward developing a BRDF-based treatment of radiative transfer through a canopy for land surface models that can realistically simulate the mean albedo and the solar zenith angle dependence of albedo.