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Wiley, Advanced Materials, 48(27), p. 8088-8094, 2015

DOI: 10.1002/adma.201502855

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Polymerized Ionic Networkswith High Charge Density: Quasi-Solid Electrolytes in Lithium Metal Batteries

This paper is available in a repository.
This paper is available in a repository.

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Abstract

Polymerized ionic networks (PINs) with six ion pairs per repeating unit are synthesized by nucleophilic-substitution-mediated polymerization or radical polymerization of monomers bearing six 1-vinylimidazolium cations. PIN-based solid-like electrolytes show good ionic conductivities (up to 5.32 × 10(-3) S cm(-1) at 22 °C), wide electrochemical stability windows (up to 5.6 V), and good interfacial compatibility with the electrodes.