Published in
Royal Society of Chemistry, Dalton Transactions, 10(52), p. 3176-3187, 2023
DOI: 10.1039/d2dt03284h
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Experimental and computational investigation of heteroatom substitution in nucleolytic Cu(ii) cyclen complexes for balancing stability and redox activity
Journal article published in 2023 by
Jan Hormann,
Olga Verbitsky,
Xiaoyu Zhou,
Beatrice Battistella 
,
Margarete van der Meer,
Biprajit Sarkar ,
Cunyuan Zhao,
Nora Kulak
,
Margarete van der Meer,
Biprajit Sarkar ,
Cunyuan Zhao,
Nora Kulak
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Abstract
Cu(ii) complexes of heteroatom-substituted cyclen-based ligands were optmizied regarding their redox activity and DNA cleavage activity. The ideal ligand exhibited a balanced set of hard and soft donors (CuL6 with N, O and S donor atoms).