Published in

American Association for the Advancement of Science, Science, 6476(367), p. 428-430, 2020

DOI: 10.1126/science.aay2474

Links

Tools

Export citation

Search in Google Scholar

Visualizing H 2 O molecules reacting at TiO 2 active sites with transmission electron microscopy

This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

Full text: Unavailable

Green circle
Preprint: archiving allowed
Green circle
Postprint: archiving allowed
Red circle
Published version: archiving forbidden
Data provided by SHERPA/RoMEO

Abstract

Imaging reactive surface water Recent developments in transmission electron microscopy (TEM) have enabled imaging of single atoms, but adsorbed gas molecules have proven more challenging because of a lack of sufficient image contrast. Yuan et al. adsorbed water and carbon monoxide (CO) on a reconstructed nanocrystalline anatase titanium dioxide (TiO 2 ) surface that has protruding TiO 3 ridges every four unit cells, which provide regions of distinct contrast. Water adsorption on this surface during environmental TEM experiments led to the formation of twinned protrusions. These structures developed dynamic contrast as the water reacted with coexposed CO to form hydrogen and carbon dioxide. Science , this issue p. 428