This experiment was aimed at verifying the usefulness of phytoremediation using Short Rotation Coppice (SRC) in an urban Zn-contaminated site. Besides elemental uptake and reclamation, the SRC method was applied to evaluate the additional benefits of a green infrastructure. Nine different plants with rapid growth and large biomass production were selected: three Populus clones, three Salix hybrids, and three Robinia genotypes. Annual and biennial coppicing were evaluated. Poplar clones were more productive using annual coppicing, while Salix and Robinia produced higher biomass in blocks not coppiced. Poplar had the highest phytoextraction rate during the second year, with 1077 g/ha. Salix clones S1 and S3 extracted similar quantities using biennial coppicing. After two years, the bioavailable fraction of Zn decreased significantly using all species, from the 26% decrease of Robinia to the 36% decrease of Salix. The short rotation coppice method proved to be useful in an urban context, for both landscape and limiting the access to the contaminated area. Improving the biomass yield through the phytomanagement options (fertilization, irrigation, coppicing, etc.) could make SRC phytoremediation an economic and effective solution to manage urban contaminated areas, coupling the added values of biomass production to the landscape benefits.