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European Geosciences Union, Geoscientific Model Development, 6(5), p. 1363-1375, 2012

DOI: 10.5194/gmd-5-1363-2012

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Modeling wet deposition and concentration of inorganics over Northeast Asia with MRI-PM/c

Journal article published in 2012 by M. Kajino, M. Deushi ORCID, T. Maki, N. Oshima, Y. Inomata, K. Sato, T. Ohizumi, H. Ueda
This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Abstract. We conducted a regional-scale simulation over Northeast Asia for the year 2006 using an aerosol chemical transport model, with time-varying lateral and upper boundary concentrations of gaseous species predicted by a global stratospheric and tropospheric chemistry-climate model. The present one-way nested global-through-regional-scale model is named the Meteorological Research Institute–Passive-tracers Model system for atmospheric Chemistry (MRI-PM/c). We evaluated the model's performance with respect to the major anthropogenic and natural inorganic components, SO42−, NH4+, NO3−, Na+ and Ca2+ in the air, rain and snow measured at the Acid Deposition Monitoring Network in East Asia (EANET) stations. Statistical analysis showed that approximately 40–50 % and 70–80 % of simulated concentration and wet deposition of SO42−, NH4+, NO3−and Ca2+ are within factors of 2 and 5 of the observations, respectively. The prediction of the sea-salt originated component Na+ was not successful at near-coastal stations (where the distance from the coast ranged from 150 to 700 m), because the model grid resolution (Δx=60 km) is too coarse to resolve it. The simulated Na+ in precipitation was significantly underestimated by up to a factor of 30.