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Nature Research, Nature Communications, 1(5), 2014

DOI: 10.1038/ncomms5953

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A room temperature low-threshold ultraviolet plasmonic nanolaser

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

Constrained by large ohmic and radiation losses, plasmonic nanolasers operated at visible regime are usually achieved either with a high threshold (10(2)-10(4) MW cm(-2)) or at cryogenic temperatures (4-120 K). Particularly, the bending-back effect of surface plasmon (SP) dispersion at high energy makes the SP lasing below 450 nm more challenging. Here we demonstrate the first strong room temperature ultraviolet (~370 nm) SP polariton laser with an extremely low threshold (~3.5 MW cm(-2)). We find that a closed-contact planar semiconductor-insulator-metal interface greatly lessens the scattering loss, and more importantly, efficiently promotes the exciton-SP energy transfer thus furnishes adequate optical gain to compensate the loss. An excitation polarization-dependent lasing action is observed and interpreted with a microscopic energy-transfer process from excitons to SPs. Our work advances the fundamental understanding of hybrid plasmonic waveguide laser and provides a solution of realizing room temperature UV nanolasers for biological applications and information technologies.