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American Physical Society, Physical review B, 13(72), 2005

DOI: 10.1103/physrevb.72.134419

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Magnetization reversal and nanoscopic magnetic-phase separation inLa1−xSrxCoO3

Journal article published in 2005 by Joseph E. Davies, J. Wu, C. Leighton, Kai Liu ORCID
This paper is available in a repository.
This paper is available in a repository.

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Abstract

The doped perovskite cobaltite La1-x Srx CoO3 (LSCO) has been advanced as a model system for studying intrinsic magnetic phase separation. We have employed a first-order reversal curve (FORC) method to probe the amount of irreversible switching in bulk polycrystalline LSCO as a function of Sr doping, field cooling procedure, and temperature. The value of the FORC distribution rho is used as a measure of the extent of irreversible switching. For x0.18 , the much larger values of rho , the tilting of its distribution towards negative bias field, and the emergence of regions with negative rho are consistent with increased long-range ferromagnetic ordering. The FORC distributions display little dependence on the cooling procedure. With increasing temperature, the fraction of irreversible switching determined from the FORC distribution follows closely the ferromagnetic phase fraction measured by La nuclear magnetic resonance. Our results furthermore demonstrate that the FORC method is a valuable first-pass characterization tool for magnetic-phase separation.