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American Physical Society, Physical Review Letters, 14(114), 2015

DOI: 10.1103/physrevlett.114.146802

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Experimental Verification of the Van Vleck Nature of Long-Range Ferromagnetic Order in the Vanadium-Doped Three-Dimensional Topological InsulatorSb2Te3

This paper is made freely available by the publisher.
This paper is made freely available by the publisher.

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Abstract

We demonstrate by high resolution low temperature electron energy loss spectroscopy (EELS) measurements that the long range ferromagnetic (FM) order in vanadium (V)-doped topological insulator Sb$_2$Te$_3$ has the nature of van Vleck-type ferromagnetism. The positions and the relative amplitudes of two core-level peaks (L$_3$ and L$_2$) of the V EELS spectrum show unambiguous change when the sample is cooled from room temperature to T=10K. Magnetotransport and comparison of the measured and simulated EELS spectra confirm that these changes originate from onset of FM order. Crystal field analysis indicates that in V-doped Sb$_2$Te$_3$, partially filled core states contribute to the FM order. Since van Vleck magnetism is a result of summing over all states, this magnetization of core level verifies the van Vleck-type ferromagnetism in a direct manner. ; Comment: 5 pages, 5 figures