Published in
Royal Society of Chemistry, Physical Chemistry Chemical Physics, 8(26), p. 6726-6735, 2024
DOI: 10.1039/d3cp05712g
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Beyond the electrical double layer model: ion-dependent effects in nanoscale solvent organization
Journal article published in 2024 by
Amanda J. Souna,
Mohammad H. Motevaselian,
Jake W. Polster 
,
Jason D. Tran,
Zuzanna S. Siwy ,
Narayana R. Aluru ,
John T. Fourkas
,
Jason D. Tran,
Zuzanna S. Siwy ,
Narayana R. Aluru ,
John T. Fourkas
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Abstract
Electrochemical measurements, nonlinear spectroscopy, and MD simulations are used to explore how the sizes and identities of ions influence their non-uniform distribution in acetonitrile that is highly organized due to proximity to a polar interface.