Published in
Royal Society of Chemistry, Nanoscale, 36(13), p. 15215-15219, 2021
DOI: 10.1039/d1nr04229g
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Power discontinuity and shift of the energy onset of a molecular de-bromination reaction induced by hot-electron tunneling
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Abstract
We describe the electron-induced dissociation of Br atoms in the Au(Br-MBP)2 complex, showing that the reaction onset can be shifted from 2.4 to 4.4 V while the required power drops sharply to 20% when a second molecular resonance is involved.