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American Institute of Physics, Applied Physics Letters, 9(122), p. 092201, 2023

DOI: 10.1063/5.0136787

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Suppression of atomic displacive excitation in photo-induced A<sub>1g</sub> phonon mode of bismuth unveiled by low-temperature time-resolved x-ray diffraction

This paper was not found in any repository, but could be made available legally by the author.
This paper was not found in any repository, but could be made available legally by the author.

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Abstract

An ultrafast atomic motion of a photo-induced coherent phonon of bismuth at low temperatures was directly observed with time-resolved x-ray diffraction. A cryostat with a window that is transparent to both optical lasers and x rays enabled versatile diffraction measurements in a wide temperature range including below 10 K. It is found that an atomic displacement in a fully symmetric A1g phonon mode is suppressed at low temperatures. This result indicates that the displacive excitation process is suppressed in the phonon generation with the decrease in temperature.