Hydrogen bonding to oxygen in siloxane bonds drives liquid phase adsorption of primary alcohols in high-silica zeolites
Journal article published in 2023 by
Sambhu Radhakrishnan 
,
Charlotte Lejaegere ,
Karel Duerinckx,
Wei-Shang Lo,
Alysson F. Morais ,
Dirk Dom,
C. Vinod Chandran ,
Ive Hermans ,
Johan A. Martens ,
Eric Breynaert
,
Charlotte Lejaegere ,
Karel Duerinckx,
Wei-Shang Lo,
Alysson F. Morais ,
Dirk Dom,
C. Vinod Chandran ,
Ive Hermans ,
Johan A. Martens ,
Eric Breynaert
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Abstract
NMR reveals alcohols and water adsorb in high silica zeolites by hydrogen bonding to siloxane bridges. This new mechanism co-exists with chemi- and physi-sorption on Brønsted acid and defect sites and drives pore filling adsorption in MFI zeolites.