Abstract With the advent of high-cadence, all-sky automated surveys, supernovae (SNe) are now discovered closer than ever to their dates of explosion. However, young premaximum light follow-up spectra of Type Ic SNe (SNe Ic), probably arising from the most-stripped massive stars, remain rare despite their importance. In this Letter, we present a set of 49 optical spectra observed with the Las Cumbres Observatory through the Global Supernova Project for 6 SNe Ic, including a total of 17 premaximum spectra, of which 8 are observed more than a week before V-band maximum light. This data set increases the total number of publicly available premaximum-light SN Ic spectra by 25%, and we provide publicly available SNID templates that will significantly aid in the fast identification of young SNe Ic in the future. We present a detailed analysis of these spectra, including Fe ii 5169 velocity measurements, O i 7774 line strengths, and continuum shapes. We compare our results to published samples of stripped SNe in the literature and find one SN in our sample that stands out. SN 2019ewu has a unique combination of features for an SN Ic: an extremely blue continuum, high absorption velocities, a P Cygni–shaped feature almost 2 weeks before maximum light that TARDIS radiative transfer modeling attributes to C ii rather than Hα, and weak or nonexistent O i 7774 absorption feature until maximum light.